I struggle to think of a smoother looking pick than Spillane’s — few things better than a backer perfectly jumping the route going in the other direction.
But off the top of my head, the best picks that come to mind recently are:
Erik Harris to seal the win against the colts: https://www.nfl.com/videos/raiders-first-int-of-19-is-pick-six-from-erik-harris
Daryl Worley was a terrible CB but probably the most remarkable INT ive ever seen: https://www.youtube.com/watch?v=xbEj_r3NgB0
Jeff Heath picking Mahomes : https://www.youtube.com/watch?v=53fPEJb1awo
Kwiatkoski’s one hander against Denver https://www.raiders.com/video/nick-kwiatkoski-intercepts-drew-lock-to-finalize-win-over-denver
Chris Carr pick 6 against Pittsburgh in 2006
Rod Woodson pick 6 in Denver on Monday Night in 2002
Khalil Mack pick 6 on Cam Newton in 2016 (I was there)
Michael Huff game winning INT in 2011 as time expired in Houston (a day after Al Davis’ death.)