I struggle to think of a smoother looking pick than Spillane’s — few things better than a backer perfectly jumping the route going in the other direction.
But off the top of my head, the best picks that come to mind recently are:
Erik Harris to seal the win against the colts: https://www.nfl.com/videos/raiders-first-int-of-19-is-pick-six-from-erik-harris
Daryl Worley was a terrible CB but probably the most remarkable INT ive ever seen: https://www.youtube.com/watch?v=xbEj_r3NgB0
Jeff Heath picking Mahomes : https://www.youtube.com/watch?v=53fPEJb1awo
Kwiatkoski’s one hander against Denver https://www.raiders.com/video/nick-kwiatkoski-intercepts-drew-lock-to-finalize-win-over-denver
David Amerson picked off Alex Smith and ran it in for a touchdown back in January of 2016. The announcers were making a big deal out of Smith’s streak of games without throwing an interception, and Amerson pointed at him while he ran by him towards the end zone.
That one stuck with me. Good times.